Biomass converted carbon quantum dots for all-weather solar cells

[Display omitted] •CQDs are converted from soybean powders by a hydrothermal method.•The biomass converted CQDs are used for all-weather DSSCs.•The so-called all-weather DSSCs can generate electricity in the daytime and dark.•A dark efficiency as high as 7.97% is determined on the all-weather photov...

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Veröffentlicht in:Electrochimica acta 2017-12, Vol.257, p.259-266
Hauptverfasser: Meng, Yuanyuan, Zhang, Yue, Sun, Weiyin, Wang, Min, He, Benlin, Chen, Haiyan, Tang, Qunwei
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Sprache:eng
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Zusammenfassung:[Display omitted] •CQDs are converted from soybean powders by a hydrothermal method.•The biomass converted CQDs are used for all-weather DSSCs.•The so-called all-weather DSSCs can generate electricity in the daytime and dark.•A dark efficiency as high as 7.97% is determined on the all-weather photovoltaics.•The launched solar cell extend our knowledge of advanced all-weather solar cells. A great challenge for state-of-the-art photovoltaic devices is to realize electric power generation in all weathers. We constructively demonstrate here the conversion from biomass to carbon quantum dots for all-weather carbon quantum dot solar cells that can generate electricity in the daytime and in the dark. The combination of green-emitting long persistence phosphors with mesoscopic titanium dioxide realizes optical storage by composite photoanode under illumination and excitation to monochromatic green light in the dark. The optimized all-weather solar cell yields maximized dark power conversion efficiency as high as 7.97% along with persistent electricity output for several hours. This work begins a photovoltaic revolution to forward all-weather solar cells as future energy solutions.
ISSN:0013-4686
1873-3859
DOI:10.1016/j.electacta.2017.10.086