Engineering the Surface Structure of MoS2 Nanosheets by Carbon-Doping with Rich Defects to Tune UV-Visible Light Absorption Property

A facile doping method utilizing inexpensive raw materials was proposed to achieve variation in optical bandgap and UV-visible light absorption property of MoS2 nanosheets. Carbon-assistant heating with degreasing cotton has demonstrated the development of carbon-doped MoS2 nanosheets with enhanced rich defects. The results obtained shown that modified MoS2 nanosheets with the lateral width of ~600 nm are exhibited shift of the intensively blue peaks of photo-luminescence (PL) comparing to those MoS2 nanosheets with a lateral dimension of larger than 1 μm. Optical bandgap of the carbon-doped MoS2 nanosheets was found to be broader than that of the pure MoS2 nanosheets and the prepared samples also exhibited a broadband UV-visible light absorption property.