Effect of Si Substitution on the Antiferromagnetic Ordering in the Kondo Semiconductor CeRu^sub 2^Al^sub 10

We have studied the effect of 3p electron doping on the unusual antiferromagnetic (AFM) order in the Kondo semiconductor ... with TN = 27 K by measuring the magnetic susceptibility ..., specific heat C, and electrical resistivity ... for polycrystalline samples of ... The large decrease in the absol...

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Veröffentlicht in:Journal of the Physical Society of Japan 2016-03, Vol.85 (3), p.1
Hauptverfasser: Hayashi, Kyosuke, Muro, Yuji, Fukuhara, Tadashi, Kawabata, Jo, Kuwai, Tomohiko, Takabatake, Toshiro
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container_title Journal of the Physical Society of Japan
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creator Hayashi, Kyosuke
Muro, Yuji
Fukuhara, Tadashi
Kawabata, Jo
Kuwai, Tomohiko
Takabatake, Toshiro
description We have studied the effect of 3p electron doping on the unusual antiferromagnetic (AFM) order in the Kondo semiconductor ... with TN = 27 K by measuring the magnetic susceptibility ..., specific heat C, and electrical resistivity ... for polycrystalline samples of ... The large decrease in the absolute value of paramagnetic Curie temperature |...P| with increasing y indicates the suppression of c-f hybridization. The thermal activation behavior in ...(T) above TN disappears for y = 0.3 and TN decreases to 12 K for y = 0.38. These systematic changes in |...P|, ...(T), and TN coincide with those reported in the 4d-electron doped system Ce(Ru1-xRhx)2Al10 with respect to the number of doped electrons per formula unit. This coincidence indicates that the Al 3p- and Ru 4d-electrons in ... play the equivalent role in both the formation of hybridization gap and the unusual AFM ordering. (ProQuest: ... denotes formulae/symbols omitted.)
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The large decrease in the absolute value of paramagnetic Curie temperature |...P| with increasing y indicates the suppression of c-f hybridization. The thermal activation behavior in ...(T) above TN disappears for y = 0.3 and TN decreases to 12 K for y = 0.38. These systematic changes in |...P|, ...(T), and TN coincide with those reported in the 4d-electron doped system Ce(Ru1-xRhx)2Al10 with respect to the number of doped electrons per formula unit. This coincidence indicates that the Al 3p- and Ru 4d-electrons in ... play the equivalent role in both the formation of hybridization gap and the unusual AFM ordering. 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The large decrease in the absolute value of paramagnetic Curie temperature |...P| with increasing y indicates the suppression of c-f hybridization. The thermal activation behavior in ...(T) above TN disappears for y = 0.3 and TN decreases to 12 K for y = 0.38. These systematic changes in |...P|, ...(T), and TN coincide with those reported in the 4d-electron doped system Ce(Ru1-xRhx)2Al10 with respect to the number of doped electrons per formula unit. This coincidence indicates that the Al 3p- and Ru 4d-electrons in ... play the equivalent role in both the formation of hybridization gap and the unusual AFM ordering. 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subjects Electrons
Hybridization
Magnetism
Polycrystals
Semiconductors
title Effect of Si Substitution on the Antiferromagnetic Ordering in the Kondo Semiconductor CeRu^sub 2^Al^sub 10
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