Effect of reaction variables on CO methanation process over NiO-La^sub 2^O3-MgO/Al^sub 2^O3 catalyst for coal to synthetic natural gas

Reaction variables for methanation process were investigated using self-independently developed NiO-La^sub 2^O3-MgO/Al^sub 2^O3 catalyst in a big lab scale reactor. The effects of reaction parameters, such as temperature, pressure, H2/CO flow ratio and space velocity on the activity of methanation c...

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Veröffentlicht in:Applied petrochemical research 2015-07, Vol.5 (4), p.413
Hauptverfasser: He, Zhong, Wang, Xiaolong, Gao, Shiwang, Xiao, Tiancun
Format: Artikel
Sprache:eng
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Zusammenfassung:Reaction variables for methanation process were investigated using self-independently developed NiO-La^sub 2^O3-MgO/Al^sub 2^O3 catalyst in a big lab scale reactor. The effects of reaction parameters, such as temperature, pressure, H2/CO flow ratio and space velocity on the activity of methanation catalyst were studied. 100 % CO conversion and 95 % of selectivity of methane can be achieved at 400 °C and 3 MPa with the feed ratio of H2/CO as 3.25:1 and space velocity of 12,000 h^sup -1^.The optimization reaction parameters were suggested on the basis of this work for the further development and commercialization of methanation catalyst.
ISSN:2190-5525
2190-5525
DOI:10.1007/s13203-015-0127-9