Phase Transfer‐Catalyzed Fast CO2 Absorption by MgO‐Based Absorbents with High Cycling Capacity
Molten salts facilitate the reaction of CO2 with MgO by providing an alternate pathway to traditional gas‐solid reactions. Molten salts partially dissolve bulk MgO and provide activated species accessible to CO2 at gas‐solid‐liquid triple phase boundaries. This methodology is also applicable to othe...
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| Veröffentlicht in: | Advanced Materials Interfaces, 1(3):Article No. 1400030 1(3):Article No. 1400030, 2014-06, Vol.1 (3), p.n/a |
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| container_title | Advanced Materials Interfaces, 1(3):Article No. 1400030 |
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| creator | Zhang, Keling Li, Xiaohong Shari Li, Wei‐Zhen Rohatgi, Aashish Duan, Yuhua Singh, Prabhakar Li, Liyu King, David L. |
| description | Molten salts facilitate the reaction of CO2 with MgO by providing an alternate pathway to traditional gas‐solid reactions. Molten salts partially dissolve bulk MgO and provide activated species accessible to CO2 at gas‐solid‐liquid triple phase boundaries. This methodology is also applicable to other basic metal oxides and molten salts, inspiring the design of new absorbent systems. |
| doi_str_mv | 10.1002/admi.201400030 |
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(PNNL), Richland, WA (United States)</creatorcontrib><description>Molten salts facilitate the reaction of CO2 with MgO by providing an alternate pathway to traditional gas‐solid reactions. Molten salts partially dissolve bulk MgO and provide activated species accessible to CO2 at gas‐solid‐liquid triple phase boundaries. This methodology is also applicable to other basic metal oxides and molten salts, inspiring the design of new absorbent systems.</description><identifier>ISSN: 2196-7350</identifier><identifier>EISSN: 2196-7350</identifier><identifier>DOI: 10.1002/admi.201400030</identifier><language>eng</language><publisher>Weinheim: John Wiley & Sons, Inc</publisher><subject>carbonate ; catalysis ; CO2 capture ; metal oxides ; molten salts ; phase transfer catalysis ; triple phase boundary ; warm temperature CO2 capture</subject><ispartof>Advanced Materials Interfaces, 1(3):Article No. 1400030, 2014-06, Vol.1 (3), p.n/a</ispartof><rights>2014 WILEY‐VCH Verlag GmbH & Co. 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(PNNL), Richland, WA (United States)</creatorcontrib><title>Phase Transfer‐Catalyzed Fast CO2 Absorption by MgO‐Based Absorbents with High Cycling Capacity</title><title>Advanced Materials Interfaces, 1(3):Article No. 1400030</title><description>Molten salts facilitate the reaction of CO2 with MgO by providing an alternate pathway to traditional gas‐solid reactions. Molten salts partially dissolve bulk MgO and provide activated species accessible to CO2 at gas‐solid‐liquid triple phase boundaries. This methodology is also applicable to other basic metal oxides and molten salts, inspiring the design of new absorbent systems.</description><subject>carbonate</subject><subject>catalysis</subject><subject>CO2 capture</subject><subject>metal oxides</subject><subject>molten salts</subject><subject>phase transfer catalysis</subject><subject>triple phase boundary</subject><subject>warm temperature CO2 capture</subject><issn>2196-7350</issn><issn>2196-7350</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><recordid>eNpNkLFOwzAQhiMEElXpymzB3HK2kzgeS6C0UqsylNlyHCdxlSYhdlWFiUfgGXkSUgUhprvT_939p9_zbjHMMAB5kOnBzAhgHwAoXHgjgnk4ZTSAy3_9tTexdt8jGBNMIjry1GshrUa7VlY20-3351csnSy7D52ihbQOxVuC5omt28aZukJJhzb5tsce-7V0UBJdOYtOxhVoafICxZ0qTZWjWDZSGdfdeFeZLK2e_Nax97Z43sXL6Xr7sorn62lOOIMplypimAV-QCQEvk5lEirCQHEWBqFPsgiilPNIypQQnnLKkzBUURho30-yJKBj7264W1tnhO2ttSpUXVVaOYExo-CzHrofoKat34_aOrGvj23V_yUwg5AA7f17ig_UyZS6E01rDrLtBAZxTluc0xZ_aYv502b1N9Efi3h1Ow</recordid><startdate>201406</startdate><enddate>201406</enddate><creator>Zhang, Keling</creator><creator>Li, Xiaohong Shari</creator><creator>Li, Wei‐Zhen</creator><creator>Rohatgi, Aashish</creator><creator>Duan, Yuhua</creator><creator>Singh, Prabhakar</creator><creator>Li, Liyu</creator><creator>King, David L.</creator><general>John Wiley & Sons, Inc</general><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>OTOTI</scope></search><sort><creationdate>201406</creationdate><title>Phase Transfer‐Catalyzed Fast CO2 Absorption by MgO‐Based Absorbents with High Cycling Capacity</title><author>Zhang, Keling ; Li, Xiaohong Shari ; Li, Wei‐Zhen ; Rohatgi, Aashish ; Duan, Yuhua ; Singh, Prabhakar ; Li, Liyu ; King, David L.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-g2970-9ac87175452a054edab6c270c9765642f808d998aad229d939b66c865e44bfb53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>carbonate</topic><topic>catalysis</topic><topic>CO2 capture</topic><topic>metal oxides</topic><topic>molten salts</topic><topic>phase transfer catalysis</topic><topic>triple phase boundary</topic><topic>warm temperature CO2 capture</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Keling</creatorcontrib><creatorcontrib>Li, Xiaohong Shari</creatorcontrib><creatorcontrib>Li, Wei‐Zhen</creatorcontrib><creatorcontrib>Rohatgi, Aashish</creatorcontrib><creatorcontrib>Duan, Yuhua</creatorcontrib><creatorcontrib>Singh, Prabhakar</creatorcontrib><creatorcontrib>Li, Liyu</creatorcontrib><creatorcontrib>King, David L.</creatorcontrib><creatorcontrib>Pacific Northwest National Lab. 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| language | eng |
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| subjects | carbonate catalysis CO2 capture metal oxides molten salts phase transfer catalysis triple phase boundary warm temperature CO2 capture |
| title | Phase Transfer‐Catalyzed Fast CO2 Absorption by MgO‐Based Absorbents with High Cycling Capacity |
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