Hydrogen Generation Using a Photoinduced Electron-transport System with a Molecular Catalyst in Vesicles

Hydrogen Generation Using a Photoinduced Electron-transport System with a Molecular Catalyst in Vesicles

We constructed a novel H2 generation system mimicking natural photosynthesis, in which an electron is transported photochemically from ascorbate entrapped in the inner waterpool of vesicles to MV2+ dissolved in the outer aqueous solution and relayed to a Pt(II) complex embedded in the vesicle membra...

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Veröffentlicht in:Chemistry letters 2011-04, Vol.40 (4), p.345-347
Hauptverfasser: Watanabe, Kentaro, Takizawa, Shin-ya, Murata, Shigeru
Format: Artikel
Sprache:eng
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Zusammenfassung:We constructed a novel H2 generation system mimicking natural photosynthesis, in which an electron is transported photochemically from ascorbate entrapped in the inner waterpool of vesicles to MV2+ dissolved in the outer aqueous solution and relayed to a Pt(II) complex embedded in the vesicle membrane that acts as a molecular catalyst.
ISSN:0366-7022
1348-0715
DOI:10.1246/cl.2011.345