Spin-charge-lattice coupling through resonant multimagnon excitations in multiferroic BiFeO{sub 3}

Spin-charge-lattice coupling mediated by multimagnon processes is demonstrated in multiferroic BiFeO{sub 3}. Experimental evidence of two- and three-magnon excitations as well as multimagnon coupling at electronic energy scales and high temperatures are reported. Temperature dependent Raman experime...

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Veröffentlicht in:Applied physics letters 2009-01, Vol.94 (2009)
Hauptverfasser: Ramirez, M. O., Kumar, A., Denev, S. A., Chu, Y. H., Seidel, J., Martin, L. W., Yang, S.-Y., Rai, R. C., Xue, X. S., Ihlefeld, J. F., Podraza, N. J., Saiz, E., Lee, S., Klug, J., Cheong, S. W., Bedzyk, M. J., Auciello, O., Schlom, D.G., Orenstein, J., Ramesh, R., Musfeldt, J. L., Litvinchuk, A. P., Gopalan, V., Pennsylvania State Univ, LBNL, Univ. California at Berkeley, Univ. Tennessee at Knoxville, The State Univ. of New Jersey, Northwestern Univ, Univ. of Houston
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Sprache:eng
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Zusammenfassung:Spin-charge-lattice coupling mediated by multimagnon processes is demonstrated in multiferroic BiFeO{sub 3}. Experimental evidence of two- and three-magnon excitations as well as multimagnon coupling at electronic energy scales and high temperatures are reported. Temperature dependent Raman experiments show up to five resonant enhancements of the two-magnon excitation below the Neel temperature. These are shown to be collective interactions between on-site Fe d-d electronic resonance, phonons, and multimagnons.
ISSN:0003-6951
1077-3118
DOI:10.1063/1.3118576