A magnetic continuum in the cobalt-based honeycomb magnet BaCo2(AsO4)2

Quantum spin liquids (QSLs) are topologically ordered states of matter that host fractionalized excitations. A particular route towards a QSL is via strongly bond-dependent interactions on the hexagonal lattice. A number of Ru- and Ir-based candidate Kitaev QSL materials have been pursued, but all have appreciable non-Kitaev interactions. Using time-domain terahertz spectroscopy, we observed a broad magnetic continuum over a wide range of temperatures and fields in the honeycomb cobalt-based magnet BaCo 2 (AsO 4 ) 2 , which has been proposed to be a more ideal version of a Kitaev QSL. Applying an in-plane magnetic field of ~0.5 T suppresses the magnetic order, and at higher fields, applying the field gives rise to a spin-polarized state. Under a 4 T magnetic field that was oriented principally out of plane, a broad magnetic continuum was observed that may be consistent with a field-induced QSL. Our results indicate BaCo 2 (AsO 4 ) 2 is a promising QSL candidate. The authors present time-domain terahertz spectroscopy measurements on BaCo 2 (AsO 4 ) 2 , a promising 3 d transition-metal-based quantum spin liquid candidate.