Evaluating the carbon footprint of the integrated DBD‐plasma bi‐reforming unit via laboratory scale experiments and scaled‐up process modeling

Abstract Catalytic dielectric barrier discharge (DBD) plasma reactor experiments were performed in a tubular glass reactor with a 2 mm gap at 550°C to facilitate the reaction kinetics of steam added dry reforming or bireforming. The best specific energy input obtained was 11.2 eV/molecule feed at CO...

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Veröffentlicht in:Plasma processes and polymers 2023-10, Vol.21 (1)
Hauptverfasser: Cao, Guoqiang, Gonzalez‐Casamachin, Diego Alexander, Xiao, Yue, Chen, Chien‐Hua, Uddi, Mruthunjaya, Baltrusaitis, Jonas
Format: Artikel
Sprache:eng
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Zusammenfassung:Abstract Catalytic dielectric barrier discharge (DBD) plasma reactor experiments were performed in a tubular glass reactor with a 2 mm gap at 550°C to facilitate the reaction kinetics of steam added dry reforming or bireforming. The best specific energy input obtained was 11.2 eV/molecule feed at CO 2 :CH 4 :H 2 O of 4.5:1:4.5 ratio and gas hour space velocity (GHSV) = 432 h −1 . This value was used to design a conceptual process and assess the environmental impact of methane steam reforming‐based H 2 production 18.4 kmol/h CO 2 emission processing into H 2 :CO = 2 syngas, with an emphasis on the carbon footprint.
ISSN:1612-8850
1612-8869