Interplay of point defects, biaxial strain, and thermal conductivity in homoepitaxial SrTiO{sub 3} thin films

Separating out effects of point defects and lattice strain on thermal conductivity is essential for improvement of thermoelectric properties of SrTiO{sub 3}. We study relations between defects generated during deposition, induced lattice strain, and their impact on thermal conductivity {kappa} in ho...

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Veröffentlicht in:Applied physics letters 2012-02, Vol.100 (6)
Hauptverfasser: Wiedigen, S., Kramer, T., Knorr, I., Nee, N., Hoffmann, J., Volkert, C. A., Jooss, Ch, Feuchter, M., Kamlah, M.
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Sprache:eng
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Zusammenfassung:Separating out effects of point defects and lattice strain on thermal conductivity is essential for improvement of thermoelectric properties of SrTiO{sub 3}. We study relations between defects generated during deposition, induced lattice strain, and their impact on thermal conductivity {kappa} in homoepitaxial SrTiO{sub 3} films prepared by ion-beam sputtering. Lowering the deposition temperature gives rise to lattice expansion by enhancement of point defect density which increases the hardness of the films. Due to a fully coherent substrate-film interface, the lattice misfit induces a large biaxial strain. However, we can show that the temperature dependence of {kappa} is mainly sensitive on the defect concentration.
ISSN:0003-6951
1077-3118
DOI:10.1063/1.3682300