High harmonic spectroscopy of multichannel dynamics in strong-field ionization

We perform high harmonic generation spectroscopy of aligned nitrogen molecules to characterize the attosecond dynamics of multielectron rearrangement during strong-field ionization. We use the spectrum and ellipticity of the harmonic light to reconstruct the relative phase between different ionizati...

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Veröffentlicht in:Physical review letters 2010-05, Vol.104 (21), p.213601-213601, Article 213601
Hauptverfasser: Mairesse, Y, Higuet, J, Dudovich, N, Shafir, D, Fabre, B, Mével, E, Constant, E, Patchkovskii, S, Walters, Z, Ivanov, M Yu, Smirnova, O
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Sprache:eng
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Zusammenfassung:We perform high harmonic generation spectroscopy of aligned nitrogen molecules to characterize the attosecond dynamics of multielectron rearrangement during strong-field ionization. We use the spectrum and ellipticity of the harmonic light to reconstruct the relative phase between different ionization continua participating in the ionization, and thus determine the shape and location of the hole left in the molecule by strong-field ionization. Our interferometric technique uses transitions between the ionic states, induced by the laser field on the subcycle time scale.
ISSN:0031-9007
1079-7114
DOI:10.1103/physrevlett.104.213601