Interference effects in IR photon echo spectroscopy of liquid water

Interference effects in IR photon echo spectroscopy of liquid water

Heterodyne-detected transient grating experiments on the OH-stretch mode of HDO dissolved in D{sub 2}O resolve two distinctly different contributions originating from the initially excited OH stretch and the OD stretch which is thermally activated during the OH population relaxation. It is demonstra...

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Veröffentlicht in:Physical review. A, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2006-02, Vol.73 (2), Article 021804
Hauptverfasser: Yeremenko, Sergey, Pshenichnikov, Maxim S., Wiersma, Douwe A.
Format: Artikel
Sprache:eng
Schlagworte:
ATOMIC AND MOLECULAR PHYSICS
HEAVY WATER
INTERFERENCE
LIQUIDS
PHOTONS
RELAXATION
SPECTROSCOPY
TRANSIENTS
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Zusammenfassung:Heterodyne-detected transient grating experiments on the OH-stretch mode of HDO dissolved in D{sub 2}O resolve two distinctly different contributions originating from the initially excited OH stretch and the OD stretch which is thermally activated during the OH population relaxation. It is demonstrated that interference of both contributions greatly affects the outcome of IR photon echo experiments.
ISSN:1050-2947
1094-1622
DOI:10.1103/PhysRevA.73.021804