Angular momentum of fission fragments in low energy fission of actinides

Independent isomeric yield ratios (IYR) of {sup 128}Sb, {sup 130}Sb, {sup 132}Sb, {sup 131}Te, {sup 133}Te, {sup 132}I, {sup 134}I, {sup 136}I, {sup 135}Xe, and {sup 138}Cs have been determined in fast neutron induced fission of {sup 232}Th, {sup 238}U, {sup 240}Pu, and {sup 244}Cm as well as in the...

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Veröffentlicht in:Physical review. C, Nuclear physics Nuclear physics, 2005-01, Vol.71 (1), Article 014304
Hauptverfasser: Naik, H., Dange, S. P., Singh, R. J.
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Sprache:eng
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Zusammenfassung:Independent isomeric yield ratios (IYR) of {sup 128}Sb, {sup 130}Sb, {sup 132}Sb, {sup 131}Te, {sup 133}Te, {sup 132}I, {sup 134}I, {sup 136}I, {sup 135}Xe, and {sup 138}Cs have been determined in fast neutron induced fission of {sup 232}Th, {sup 238}U, {sup 240}Pu, and {sup 244}Cm as well as in thermal neutron induced fission of {sup 232}U and {sup 238}Pu using radiochemical and offline {gamma}-ray spectrometric techniques. From the IYR, fragment angular momenta (J{sub rms}) have been deduced using a spin-dependent statistical model analysis. These data along with the literature data for {sup 230}Th*, {sup 234}U*, {sup 236}U*, {sup 240}Pu*, {sup 242}Pu*, {sup 244}Cm(SF), {sup 246}Cm*, {sup 250}Cf*, and {sup 252}Cf(SF) for fifteen even-Z fissioning systems show the following important features: (i) The J{sub rms} of the odd-Z fission products are higher than those of the even-Z fission products, indicating the odd-even effect. For both the odd-Z and even-Z fission products, the J{sub rms} increase with Z{sub F}{sup 2}/A{sub F}. (ii) The J{sub rms} of fragments with spherical 50-p and 82-n shells are lower compared to those of fragments outside the spherical shell, indicating the effect of shell closure proximity. (iii) The J{sub rms} of the fission products increase with mass number in spite of fluctuations in shell closure proximity and odd-even effects but do not show any correlation with the neutron emission curve. (iv) In all fifteen even-Z fissioning systems from Th to Cf, the yield-weighted J{sub rms} values show an anticorrelation with the elemental yields. (v) The odd-even fluctuation on J{sub rms} does not change drastically from Th to Cf, unlike the proton odd-even effect ({delta}{sub p}) which decreases significantly with the increase of Coulomb parameter (Z{sub F}{sup 2}/A{sub F}{sup 1/3})
ISSN:0556-2813
1089-490X
DOI:10.1103/PhysRevC.71.014304