Coherent control of strong field multiphoton absorption in the presence of dynamic Stark shifts

We show that coherent control of multiphoton transitions is possible in the strong field limit, even in the presence of large dynamic Stark shifts. By tailoring the phase of an ultrafast laser pulse, one can compensate for the dynamic Stark shift during the atom-field interaction to achieve efficien...

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Veröffentlicht in:Physical review. A, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2005-01, Vol.71 (1), Article 013423
Hauptverfasser: Trallero-Herrero, C., Cardoza, D., Weinacht, T. C., Cohen, J. L.
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Sprache:eng
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Zusammenfassung:We show that coherent control of multiphoton transitions is possible in the strong field limit, even in the presence of large dynamic Stark shifts. By tailoring the phase of an ultrafast laser pulse, one can compensate for the dynamic Stark shift during the atom-field interaction to achieve efficient population transfer in two-photon absorption. Numerical simulations for atomic sodium reveal efficient population transfer from the vertical bar 3s> ground state to the vertical bar 4s> excited state using an appropriately shaped ultrafast laser pulse. The theory and simulations provide insight into coherent control of more complicated multiphoton processes.
ISSN:1050-2947
1094-1622
DOI:10.1103/PhysRevA.71.013423