Revision of forensics-relevant nuclear data in Sb127 β decay

With a half-life of 3.85(5) d, the fission product 127Sb is potentially useful for the characterization of fallout debris that would be collected for forensic analysis following a hypothetical nuclear event. The β decay of 127Sb has many characteristic $\gamma$-ray lines, however, the majority of de...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Physical review. C 2019-03, Vol.99 (3)
Hauptverfasser: Bucher, B., Snow, M. S., Cardenas, E. S., Carney, K. P., Finck, M. R., Horkley, J. J., Kinlaw, M. T., May, E. M., Pfeiffer, J. K., Ward, J. L.
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:With a half-life of 3.85(5) d, the fission product 127Sb is potentially useful for the characterization of fallout debris that would be collected for forensic analysis following a hypothetical nuclear event. The β decay of 127Sb has many characteristic $\gamma$-ray lines, however, the majority of decay strength is concentrated in the three strongest lines near 686, 473, and 784 keV, based on low-precision spectroscopic measurements from decades ago. In a new measurement of 127Sb β decay, obtained from radiochemical separations of U photofission products, we show that the energies of the 686 and 784 lines are actually shifted lower by 0.8 and 1.1 keV, respectively. Such large discrepancies in the nuclear data inhibit accurate isotopic analyses and have important implications, for example, on the assessment of fission debris that might be collected in the days following a nuclear event. Therefore, a new evaluation of 127Sb β decay and appropriate revision to the various nuclear databases are warranted. This work reports a new set of $\gamma$-ray energies and relative intensities corresponding to 127Sb decay.
ISSN:2469-9985
2469-9993