Dimensionality-Induced Change in Topological Order in Multiferroic Oxide Superlattices

We construct ferroelectric (LuFeO_{3})_{m}/(LuFe_{2}O_{4}) superlattices with varying index m to study the effect of confinement on topological defects. We observe a thickness-dependent transition from neutral to charged domain walls and the emergence of fractional vortices. In thin LuFeO_{3} layers...

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Veröffentlicht in:Physical review letters 2021-04, Vol.126 (15), p.157601-157601, Article 157601
Hauptverfasser: Holtz, Megan E, Padgett, Elliot S, Steinhardt, Rachel, Brooks, Charles M, Meier, Dennis, Schlom, Darrell G, Muller, David A, Mundy, Julia A
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Sprache:eng
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Zusammenfassung:We construct ferroelectric (LuFeO_{3})_{m}/(LuFe_{2}O_{4}) superlattices with varying index m to study the effect of confinement on topological defects. We observe a thickness-dependent transition from neutral to charged domain walls and the emergence of fractional vortices. In thin LuFeO_{3} layers, the volume fraction of domain walls grows, lowering the symmetry from P6_{3}cm to P3c1 before reaching the nonpolar P6_{3}/mmc state, analogous to the group-subgroup sequence observed at the high-temperature ferroelectric to paraelectric transition. Our study shows how dimensional confinement stabilizes textures beyond those in bulk ferroelectric systems.
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.126.157601