Aerosols consistently suppress the convective boundary layer development

Aerosols with different vertical distribution and various optical properties induce diverse heating rates and thereby affecting convective boundary layer (CBL) development. Our results showed consistent CBL-suppression of aerosols during daytime with numerical experiments, in which aerosols were spe...

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Veröffentlicht in:Atmospheric research 2022-05, Vol.269, p.106032, Article 106032
Hauptverfasser: Zhang, Xiaoyan, Cai, Changjie, Hu, Xiao-Ming, Gao, Lan, Xu, Xiyan, Hu, Jun, Chen, Haishan
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Sprache:eng
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Zusammenfassung:Aerosols with different vertical distribution and various optical properties induce diverse heating rates and thereby affecting convective boundary layer (CBL) development. Our results showed consistent CBL-suppression of aerosols during daytime with numerical experiments, in which aerosols were specified at different heights with synthesized single scattering albedo from 64 studies and asymmetry factor from 20 studies globally. Absorbing aerosols concentrated below but close to the CBL top had the strongest suppression effect on CBL development relative to that concentrated near surface or above CBL. Aerosol cooling effect by attenuating incident solar radiation and surface heat flux exceeded its warming effect by reheating the atmosphere layer with absorbed shortwave radiation, and eventually declined net heating rate, which inhibited CBL development, lowered mixed-layer potential temperature and stabilized atmospheric stratification. Stove effect of absorbing aerosols (CBL enhancement) under a zero background aerosol extinction coefficient is negligible for dominant dome effect (CBL suppression) which consistently suppresses CBL development regardless of aerosol vertical height and background aerosol extinction coefficient. Our study also highlighted the importance of specifying background aerosol extinction coefficient in numerical experiments for accurate assessment of aerosol radiative forcing and CBL-aerosol interactions. [Display omitted] •Aerosols always suppress convective boundary layer (CBL) development.•The strongest suppression occurs when absorbing aerosols are below but near CBL top.•Aerosols reduced net heating causing lowered CBL height and enhanced stratification.•Stove effect under a zero background aerosol extinction coefficient is negligible.•Background extinction coefficient is necessary in estimating aerosol radiative effect.
ISSN:0169-8095
1873-2895
DOI:10.1016/j.atmosres.2022.106032