Large-scale dissolution of sintered Mo disks

Non-uranium production of 99 Mo via neutron capture or by photonuclear reaction using an electron accelerator is receiving considerable attention. For commercial production of 99 Mo, post-irradiation processes must incorporate a robust design for easy scale-up. Once developed, large-scale chemical p...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Journal of radioanalytical and nuclear chemistry 2021-02, Vol.327 (2), p.617-626
Hauptverfasser: Tkac, Peter, Rotsch, David A., Chemerisov, Sergey D., Byrnes, James P., Bailey, James L., Wiedmeyer, Stanley G.
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:Non-uranium production of 99 Mo via neutron capture or by photonuclear reaction using an electron accelerator is receiving considerable attention. For commercial production of 99 Mo, post-irradiation processes must incorporate a robust design for easy scale-up. Once developed, large-scale chemical processes must be optimized for hot-cell operations and potential automation. Here we present experimental results on the large-scale dissolution of sintered Mo disks using three 50% hydrogen peroxides from different suppliers. Dissolution rates obtained for 600-g Mo batches and potential reasons for different dissolution behaviors is discussed.
ISSN:0236-5731
1588-2780
DOI:10.1007/s10967-020-07566-y