Alignment of Cellulose Nanofibers: Harnessing Nanoscale Properties to Macroscale Benefits

In nature, cellulose nanofibers form hierarchical structures across multiple length scales to achieve high-performance properties and different functionalities. Cellulose nanofibers, which are separated from plants or synthesized biologically, are being extensively investigated and processed into di...

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Veröffentlicht in:ACS nano 2021-03, Vol.15 (3), p.3646-3673
Hauptverfasser: Li, Kai, Clarkson, Caitlyn M, Wang, Lu, Liu, Yu, Lamm, Meghan, Pang, Zhenqian, Zhou, Yubing, Qian, Ji, Tajvidi, Mehdi, Gardner, Douglas J, Tekinalp, Halil, Hu, Liangbing, Li, Teng, Ragauskas, Arthur J, Youngblood, Jeffrey P, Ozcan, Soydan
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container_title ACS nano
container_volume 15
creator Li, Kai
Clarkson, Caitlyn M
Wang, Lu
Liu, Yu
Lamm, Meghan
Pang, Zhenqian
Zhou, Yubing
Qian, Ji
Tajvidi, Mehdi
Gardner, Douglas J
Tekinalp, Halil
Hu, Liangbing
Li, Teng
Ragauskas, Arthur J
Youngblood, Jeffrey P
Ozcan, Soydan
description In nature, cellulose nanofibers form hierarchical structures across multiple length scales to achieve high-performance properties and different functionalities. Cellulose nanofibers, which are separated from plants or synthesized biologically, are being extensively investigated and processed into different materials owing to their good properties. The alignment of cellulose nanofibers is reported to significantly influence the performance of cellulose nanofiber-based materials. The alignment of cellulose nanofibers can bridge the nanoscale and macroscale, bringing enhanced nanoscale properties to high-performance macroscale materials. However, compared with extensive reviews on the alignment of cellulose nanocrystals, reviews focusing on cellulose nanofibers are seldom reported, possibly because of the challenge of aligning cellulose nanofibers. In this review, the alignment of cellulose nanofibers, including cellulose nanofibrils and bacterial cellulose, is extensively discussed from different aspects of the driving force, evaluation, strategies, properties, and applications. Future perspectives on challenges and opportunities in cellulose nanofiber alignment are also briefly highlighted.
doi_str_mv 10.1021/acsnano.0c07613
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source ACS Publications
subjects anisotropic properties
bacterial cellulose
cellulose nanofiber
cellulose nanofibrils
fiber alignment
functional materials
INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
nanocellulose
nanocellulose self-assembly
title Alignment of Cellulose Nanofibers: Harnessing Nanoscale Properties to Macroscale Benefits
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