Enabling high repetition rate nonlinear THz science with a kilowatt-class sub-100 fs laser source

Manipulating the atomic and electronic structure of matter with strong terahertz (THz) fields while probing the response with ultrafast pulses at x-ray free electron lasers (FELs) has offered unique insights into a multitude of physical phenomena in solid state and atomic physics. Recent upgrades of...

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Veröffentlicht in:Optics express 2020-05, Vol.28 (11), p.16951-16967
Hauptverfasser: Kramer, Patrick L., Windeler, Matthew K. R., Mecseki, Katalin, Champenois, Elio G., Hoffmann, Matthias C., Tavella, Franz
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Sprache:eng
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Zusammenfassung:Manipulating the atomic and electronic structure of matter with strong terahertz (THz) fields while probing the response with ultrafast pulses at x-ray free electron lasers (FELs) has offered unique insights into a multitude of physical phenomena in solid state and atomic physics. Recent upgrades of x-ray FEL facilities are pushing to much higher repetition rates, enabling unprecedented signal-to-noise ratio for pump probe experiments. This requires the development of suitable THz pump sources that are able to deliver intense pulses at compatible repetition rates. Here we present a high-power laser-driven THz source based on optical rectification in LiNbO 3 using tilted pulse front pumping. Our source is driven by a kilowatt-level Yb:YAG amplifier system operating at 100 kHz repetition rate and employing nonlinear spectral broadening and recompression to achieve sub-100 fs pulses with pulse energies up to 7 mJ that are necessary for high THz conversion efficiency and peak field strength. We demonstrate a maximum of 144 mW average THz power (1.44 μ J pulse energy), consisting of single-cycle pulses centered at 0.6 THz with a peak electric field strength exceeding 150 kV/cm. These high field pulses open up a range of possibilities for nonlinear time-resolved THz experiments at unprecedented rates.
ISSN:1094-4087
1094-4087
DOI:10.1364/OE.389653