Efficient, stable silicon tandem cells enabled by anion-engineered wide-bandgap perovskites
Maximizing the power conversion efficiency (PCE) of perovskite/silicon tandem solar cells that can exceed the Shockley-Queisser single-cell limit requires a high-performing, stable perovskite top cell with a wide bandgap. We developed a stable perovskite solar cell with a bandgap of ~1.7 electron vo...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2020-04, Vol.368 (6487), p.155-160 |
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| creator | Kim, Daehan Jung, Hee Joon Park, Ik Jae Larson, Bryon W Dunfield, Sean P Xiao, Chuanxiao Kim, Jekyung Tong, Jinhui Boonmongkolras, Passarut Ji, Su Geun Zhang, Fei Pae, Seong Ryul Kim, Minkyu Kang, Seok Beom Dravid, Vinayak Berry, Joseph J Kim, Jin Young Zhu, Kai Kim, Dong Hoe Shin, Byungha |
| description | Maximizing the power conversion efficiency (PCE) of perovskite/silicon tandem solar cells that can exceed the Shockley-Queisser single-cell limit requires a high-performing, stable perovskite top cell with a wide bandgap. We developed a stable perovskite solar cell with a bandgap of ~1.7 electron volts that retained more than 80% of its initial PCE of 20.7% after 1000 hours of continuous illumination. Anion engineering of phenethylammonium-based two-dimensional (2D) additives was critical for controlling the structural and electrical properties of the 2D passivation layers based on a lead iodide framework. The high PCE of 26.7% of a monolithic two-terminal wide-bandgap perovskite/silicon tandem solar cell was made possible by the ideal combination of spectral responses of the top and bottom cells. |
| doi_str_mv | 10.1126/science.aba3433 |
| format | Article |
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stable silicon tandem cells enabled by anion-engineered wide-bandgap perovskites</title><author>Kim, Daehan ; Jung, Hee Joon ; Park, Ik Jae ; Larson, Bryon W ; Dunfield, Sean P ; Xiao, Chuanxiao ; Kim, Jekyung ; Tong, Jinhui ; Boonmongkolras, Passarut ; Ji, Su Geun ; Zhang, Fei ; Pae, Seong Ryul ; Kim, Minkyu ; Kang, Seok Beom ; Dravid, Vinayak ; Berry, Joseph J ; Kim, Jin Young ; Zhu, Kai ; Kim, Dong Hoe ; Shin, Byungha</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c459t-5bea69689935381b091d40bd65db2ad50043cce90b9199d3a36b90419189ac033</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Additives</topic><topic>Anions</topic><topic>Bromine</topic><topic>Efficiency</topic><topic>Electrical properties</topic><topic>Illumination</topic><topic>Iodides</topic><topic>Iodine</topic><topic>Perovskites</topic><topic>Photovoltaic cells</topic><topic>Silicon</topic><topic>Solar 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| fulltext | fulltext |
| identifier | ISSN: 0036-8075 |
| ispartof | Science (American Association for the Advancement of Science), 2020-04, Vol.368 (6487), p.155-160 |
| issn | 0036-8075 1095-9203 |
| language | eng |
| recordid | cdi_osti_scitechconnect_1615092 |
| source | American Association for the Advancement of Science |
| subjects | Additives Anions Bromine Efficiency Electrical properties Illumination Iodides Iodine Perovskites Photovoltaic cells Silicon Solar cells |
| title | Efficient, stable silicon tandem cells enabled by anion-engineered wide-bandgap perovskites |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-18T19%3A03%3A03IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Efficient,%20stable%20silicon%20tandem%20cells%20enabled%20by%20anion-engineered%20wide-bandgap%20perovskites&rft.jtitle=Science%20(American%20Association%20for%20the%20Advancement%20of%20Science)&rft.au=Kim,%20Daehan&rft.date=2020-04-10&rft.volume=368&rft.issue=6487&rft.spage=155&rft.epage=160&rft.pages=155-160&rft.issn=0036-8075&rft.eissn=1095-9203&rft_id=info:doi/10.1126/science.aba3433&rft_dat=%3Cproquest_osti_%3E2383658504%3C/proquest_osti_%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2383658504&rft_id=info:pmid/32217753&rfr_iscdi=true |