pH Oscillator Stretched in Space but Frozen in Time

Chemical oscillations are studied using a continuous-flow microfluidic system transforming the time domain of chemical oscillators into a spatial domain. This system allows one (i) to monitor the dynamics of chemical oscillators with the accuracy of vigorously stirred batch reactors but with the eas...

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Veröffentlicht in:	The journal of physical chemistry letters 2015-03, Vol.6 (5), p.760-766
Hauptverfasser:	Hermans, Thomas M, Stewart, Peter S, Grzybowski, Bartosz A
Format:	Artikel
Sprache:	eng
Schlagworte:	catalysis (homogeneous), solar (photovoltaic), bio-inspired, charge transport, mesostructured materials, materials and chemistry by design, synthesis (novel materials), synthesis (self-assembly) Computer Simulation - utilization Electrochemistry - methods Kinetics Nickel Nonlinear Dynamics Spectrophotometry - methods Time Factors
Online-Zugang:	Volltext
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Beschreibung
Zusammenfassung:	Chemical oscillations are studied using a continuous-flow microfluidic system transforming the time domain of chemical oscillators into a spatial domain. This system allows one (i) to monitor the dynamics of chemical oscillators with the accuracy of vigorously stirred batch reactors but with the ease and speed of CSTRs and (ii) to rapidly screen the phase space of chemical oscillators in just one experiment versus a traditional series of batch measurements.
ISSN:	1948-7185 1948-7185
DOI:	10.1021/jz502711c