Transport of Europium Colloids in Vadose Zone Lysimeters at the Semiarid Hanford Site

The objective of this study was to quantify transport of Eu colloids in the vadose zone at the semiarid Hanford site. Eu-hydroxy-carbonate colloids, Eu(OH)(CO3), were applied to the surface of field lysimeters, and migration of the colloids through the sediments was monitored using wick samplers. Th...

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Veröffentlicht in:Environmental science & technology 2013-03, Vol.47 (5), p.2153-2160
Hauptverfasser: Liu, Ziru, Flury, Markus, Zhang, Z. Fred, Harsh, James B, Gee, Glendon W, Strickland, Chris E, Clayton, Ray E
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Sprache:eng
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Zusammenfassung:The objective of this study was to quantify transport of Eu colloids in the vadose zone at the semiarid Hanford site. Eu-hydroxy-carbonate colloids, Eu(OH)(CO3), were applied to the surface of field lysimeters, and migration of the colloids through the sediments was monitored using wick samplers. The lysimeters were exposed to natural precipitation (145–231 mm/year) or artificial irrigation (124–348 mm/year). Wick outflow was analyzed for Eu concentrations, supplemented by electron microscopy and energy-dispersive X-ray analysis. Small amounts of Eu colloids (
ISSN:0013-936X
1520-5851
DOI:10.1021/es304383d