Strain-Driven Oxygen Deficiency in Self-Assembled, Nanostructured, Composite Oxide Films

Oxide self-assembly is a promising bottom-up approach for fabricating new composite materials at the nanometer length scale. Tailoring the properties of such systems for a wide range of electronic applications depends on the fundamental understanding of the interfaces between the constituent phases....

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:ACS nano 2011-06, Vol.5 (6), p.4783-4789
Hauptverfasser: Cantoni, Claudia, Gao, Yanfei, Wee, Sung Hun, Specht, Eliot D, Gazquez, Jaume, Meng, Jianyong, Pennycook, Stephen J, Goyal, Amit
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:Oxide self-assembly is a promising bottom-up approach for fabricating new composite materials at the nanometer length scale. Tailoring the properties of such systems for a wide range of electronic applications depends on the fundamental understanding of the interfaces between the constituent phases. We show that the nanoscale strain modulation in self-assembled systems made of high-T c superconducting films containing nanocolumns of BaZrO3 strongly affects the oxygen composition of the superconductor. Our findings explain the observed reduction of the superconducting critical temperature.
ISSN:1936-0851
1936-086X
DOI:10.1021/nn2007628