Direct Experimental Observation of Harmonics of Josephson Generation in the Flux-Flow Oscillator

We present an experimental observation and a study of harmonics of radiation from a flux-flow oscillator (FFO) based on a long Josephson junction. An integrated microcircuit consisting of the FFO, the transmitting antenna and a harmonic mixer (HM) was used to provide the phase-locked emission in the terahertz (THz) range to open space. Both the FFO and the HM were made of superconductor-insulator-superconductor (SIS) trilayers based on Nb/AlO x /Nb. Two independent techniques were used for detecting of the output emission: a THz Fourier transform spectrometer with a wideband detector based on an 4.2 K silicon bolometer, and a THz spectrometer based on the heterodyne SIS receiver with a high spectral resolution. The FFO spectral composition obtained using the FTS demonstrates the main Josephson frequency and clear higher harmonics. Following that, the spectral characteristics of the 2 nd harmonic at a frequency of 600-670 GHz (corresponding to the main frequency of 300-335 GHz) were carefully studied with a spectral resolution better than 0.1 MHz using the SIS receiver. To our knowledge, this is the first direct high-frequency observation of Josephson harmonics carried out at the true frequency of oscillations, which is in contrast to dc measurements.