Interfacial Dzyaloshinskii-Moriya interaction in perpendicularly magnetized Pt/Co/AlOx ultrathin films measured by Brillouin light spectroscopy

Spin waves in perpendicularly magnetized Pt/Co/AlOx/Pt ultrathin films with varying Co thicknesses (0.6-1.2 nm) have been studied with Brillouin light spectroscopy in the Damon-Eshbach geometry. The measurements reveal a pronounced nonreciprocal propagation, which increases with decreasing Co thickness. This nonreciprocity, attributed to an interfacial Dzyaloshinskii-Moriya interaction (DMI), is significantly stronger than asymmetries resulting from surface anisotropies for such modes. Results are consistent with an interfacial DMI constant Ds = - 1.7 ± 0.11pJ/m, which favors left-handed chiral spin structures. This suggests that such films below 1 nm in thickness should support chiral states such as skyrmions at room temperature.