High-Mobility, Wet-Transferred Graphene Grown by Chemical Vapor Deposition

We report high room-temperature mobility in single-layer graphene grown by chemical vapor deposition (CVD) after wet transfer on SiO2 and hexagonal boron nitride (hBN) encapsulation. By removing contaminations, trapped at the interfaces between single-crystal graphene and hBN, we achieve mobilities...

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Veröffentlicht in:ACS nano 2019-08, Vol.13 (8), p.8926-8935
Hauptverfasser: De Fazio, Domenico, Purdie, David G, Ott, Anna K, Braeuninger-Weimer, Philipp, Khodkov, Timofiy, Goossens, Stijn, Taniguchi, Takashi, Watanabe, Kenji, Livreri, Patrizia, Koppens, Frank H. L, Hofmann, Stephan, Goykhman, Ilya, Ferrari, Andrea C, Lombardo, Antonio
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Sprache:eng
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Zusammenfassung:We report high room-temperature mobility in single-layer graphene grown by chemical vapor deposition (CVD) after wet transfer on SiO2 and hexagonal boron nitride (hBN) encapsulation. By removing contaminations, trapped at the interfaces between single-crystal graphene and hBN, we achieve mobilities up to ∼70000 cm2 V–1 s–1 at room temperature and ∼120 000 cm2 V–1 s–1 at 9K. These are more than twice those of previous wet-transferred graphene and comparable to samples prepared by dry transfer. We also investigate the combined approach of thermal annealing and encapsulation in polycrystalline graphene, achieving room-temperature mobilities of ∼30 000 cm2 V–1 s–1. These results show that, with appropriate encapsulation and cleaning, room-temperature mobilities well above 10 000 cm2 V–1 s–1 can be obtained in samples grown by CVD and transferred using a conventional, easily scalable PMMA-based wet approach.
ISSN:1936-0851
1936-086X
DOI:10.1021/acsnano.9b02621