Electronic structure of the highly conductive perovskite oxide SrMoO 3

We use angle-resolved photoemission to map the Fermi surface and quasiparticle dispersion of bulklike thin films of SrMoO3 grown by pulsed laser deposition. The electronic self-energy deduced from our data reveals weak to moderate correlations in SrMoO3, consistent with our observation of well-defin...

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Veröffentlicht in:Physical review materials 2022-07, Vol.6 (7), Article 075002
Hauptverfasser: Cappelli, E., Hampel, A., Chikina, A., Guedes, E. Bonini, Gatti, G., Hunter, A., Issing, J., Biskup, N., Varela, M., Dreyer, C. E., Tamai, A., Georges, A., Bruno, F. Y., Radovic, M., Baumberger, F.
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Sprache:eng
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Zusammenfassung:We use angle-resolved photoemission to map the Fermi surface and quasiparticle dispersion of bulklike thin films of SrMoO3 grown by pulsed laser deposition. The electronic self-energy deduced from our data reveals weak to moderate correlations in SrMoO3, consistent with our observation of well-defined electronic states over the entire occupied bandwidth. We further introduce spectral function calculations that combine dynamical mean-field theory with an unfolding procedure of density functional calculations and demonstrate good agreement of this approach with our experiments.
ISSN:2475-9953
2475-9953
DOI:10.1103/PhysRevMaterials.6.075002