Dispersion of Molecular Patterns Written in Turbulent Air

We study the dispersion of tiny molecular clouds in turbulence by writing patterns in turbulent air and following their deformation in time. The writing is done by fusing O_{2} and N_{2} molecules into NO in the focus of a strong ultraviolet laser beam. By crossing several of these laser beams, patt...

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Veröffentlicht in:Physical review letters 2022-12, Vol.129 (25), p.254501-254501, Article 254501
Hauptverfasser: van de Water, Willem, Dam, Nico, Calzavarini, Enrico
Format: Artikel
Sprache:eng
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Zusammenfassung:We study the dispersion of tiny molecular clouds in turbulence by writing patterns in turbulent air and following their deformation in time. The writing is done by fusing O_{2} and N_{2} molecules into NO in the focus of a strong ultraviolet laser beam. By crossing several of these laser beams, patterns that have both small and large scales can be painted. The patterns are visualized a while later by inducing fluorescence of the NO molecules with a second UV laser and registering the image. The width of the lines that make the pattern is approximately 50  μm, a few times the Kolmogorov length η, the smallest length scale in turbulence, while the overall size of the patterns (≈4  mm) is inside the inertial range of the used turbulent jet flow. At small scales molecular clouds disperse under the joint action of molecular diffusion and turbulence. The experiments reveal for the first time this subtle, yet very important interaction. At macroscales (≈200  η) we verify the Batchelor dispersion of objects whose size is inside the inertial range; however, the expected influence of molecular diffusion is smaller than the accuracy of the experiments.
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.129.254501