Boosting the Catalytic Activity and Stability of Ru Metal Clusters in Hydrodeoxygenation of Guaiacol through MWW Zeolite Pore Constraints

Liquid-phase hydrodeoxygenation (HDO), catalyzed by metal or metal-acid sites, provides an effective catalytic strategy to remove oxygen-containing functionalities of lignin-derived phenolic compounds on the route to fuels and chemicals. Developing the catalyst with high activity and stability is cr...

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Veröffentlicht in:ACS catalysis 2022-12, Vol.12 (23), p.14717-14726
Hauptverfasser: He, Ping, Yi, Qisong, Geng, Huawei, Shao, Yuanchao, Liu, Meng, Wu, Zhijie, Luo, Wenhao, Liu, Yuanshuai, Valtchev, Valentin
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Sprache:eng
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Zusammenfassung:Liquid-phase hydrodeoxygenation (HDO), catalyzed by metal or metal-acid sites, provides an effective catalytic strategy to remove oxygen-containing functionalities of lignin-derived phenolic compounds on the route to fuels and chemicals. Developing the catalyst with high activity and stability is crucial for such a chemical process but still remains a significant challenge. In this contribution, highly dispersed subnanometric Ru metal clusters (
ISSN:2155-5435
2155-5435
DOI:10.1021/acscatal.2c04597