Quantification of curium isotopes in environmental samples: drawbacks, speciation and specific tracer
In this study, drawbacks of the use of 243 Am as a tracer in order to quantify curium isotopes during a complex chemical procedure were highlighted. These drawbacks were investigated through a speciation computation simulation based on the compilation of over 50 stability constants. A new curium sta...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2021-08, Vol.329 (2), p.545-554 |
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| container_end_page | 554 |
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| container_issue | 2 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
| container_volume | 329 |
| creator | Habibi, Azza Le Corre, Roselyne Wampach Aubert, Christèle Fleury, Sandrine Hennequet, Patricia Augeray, Céline Galliez, Kévin Agarande, Michelle |
| description | In this study, drawbacks of the use of
243
Am as a tracer in order to quantify curium isotopes during a complex chemical procedure were highlighted. These drawbacks were investigated through a speciation computation simulation based on the compilation of over 50 stability constants. A new curium standard was then characterized and used to quantify a wide
244
Cm activities range in environmental samples. Obtained results were in excellent agreement with spiked activities and more consistent than those obtained when using
243
Am as tracer. |
| doi_str_mv | 10.1007/s10967-021-07751-7 |
| format | Article |
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243
Am as a tracer in order to quantify curium isotopes during a complex chemical procedure were highlighted. These drawbacks were investigated through a speciation computation simulation based on the compilation of over 50 stability constants. A new curium standard was then characterized and used to quantify a wide
244
Cm activities range in environmental samples. Obtained results were in excellent agreement with spiked activities and more consistent than those obtained when using
243
Am as tracer.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-021-07751-7</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Chemical Sciences ; Chemistry ; Chemistry and Materials Science ; Curium isotopes ; Diagnostic Radiology ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; Isotopes ; Nuclear Chemistry ; Nuclear energy ; Nuclear fuel cycle ; Nuclear industry ; Nuclear Physics ; Physical Chemistry ; Speciation ; Stability constants ; Tracers (Biology)</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2021-08, Vol.329 (2), p.545-554</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2021</rights><rights>COPYRIGHT 2021 Springer</rights><rights>Akadémiai Kiadó, Budapest, Hungary 2021.</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c436t-5a94bd26df189d9ba1bb034aace83f440f8df99a370c1a584391944cc5c290673</citedby><cites>FETCH-LOGICAL-c436t-5a94bd26df189d9ba1bb034aace83f440f8df99a370c1a584391944cc5c290673</cites><orcidid>0000-0002-8041-2990 ; 0000-0003-3829-7842</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-021-07751-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-021-07751-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>230,314,778,782,883,27907,27908,41471,42540,51302</link.rule.ids><backlink>$$Uhttps://hal.science/hal-03368652$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Habibi, Azza</creatorcontrib><creatorcontrib>Le Corre, Roselyne</creatorcontrib><creatorcontrib>Wampach Aubert, Christèle</creatorcontrib><creatorcontrib>Fleury, Sandrine</creatorcontrib><creatorcontrib>Hennequet, Patricia</creatorcontrib><creatorcontrib>Augeray, Céline</creatorcontrib><creatorcontrib>Galliez, Kévin</creatorcontrib><creatorcontrib>Agarande, Michelle</creatorcontrib><title>Quantification of curium isotopes in environmental samples: drawbacks, speciation and specific tracer</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>In this study, drawbacks of the use of
243
Am as a tracer in order to quantify curium isotopes during a complex chemical procedure were highlighted. These drawbacks were investigated through a speciation computation simulation based on the compilation of over 50 stability constants. A new curium standard was then characterized and used to quantify a wide
244
Cm activities range in environmental samples. Obtained results were in excellent agreement with spiked activities and more consistent than those obtained when using
243
Am as tracer.</description><subject>Chemical Sciences</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Curium isotopes</subject><subject>Diagnostic Radiology</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inorganic Chemistry</subject><subject>Isotopes</subject><subject>Nuclear Chemistry</subject><subject>Nuclear energy</subject><subject>Nuclear fuel cycle</subject><subject>Nuclear industry</subject><subject>Nuclear Physics</subject><subject>Physical Chemistry</subject><subject>Speciation</subject><subject>Stability constants</subject><subject>Tracers (Biology)</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNp9kU9rFTEUxYNY8Fn9Aq4GXAlOezP57-5R1AoPSkHXIZNJaupMMiYzlX57M47ormQRcjnnd084CL3BcIEBxGXBoLhoocMtCMFwK56hA2ZStp2Q8BwdoCO8ZYLgF-hlKfcAoKQkB-RuVxOX4IM1S0ixSb6xaw7r1ISSljS70oTYuPgQcoqTi4sZm2KmeXTlQzNk86s39kd535TZ2bAjTBz2Z4U2SzbW5VfozJuxuNd_73P07dPHr1fX7enm85er46m1lPClZUbRfuj44LFUg-oN7nsg1FSEJJ5S8HLwShkiwGLDJCUKK0qtZbZTwAU5R-927ncz6jmHyeRHnUzQ18eT3mZACJecdQ-4at_u2jmnn6sri75Pa441nu4Y4xQU0I14savuzOh0iD5tP6pncFOwKTof6vzIBWCOKSXV0O0Gm1Mp2fl_OTDorSu9d6VrV_pPV3rbQnZTqeJ45_L_LE-4fgM8dJcj</recordid><startdate>20210801</startdate><enddate>20210801</enddate><creator>Habibi, Azza</creator><creator>Le Corre, Roselyne</creator><creator>Wampach Aubert, Christèle</creator><creator>Fleury, Sandrine</creator><creator>Hennequet, Patricia</creator><creator>Augeray, Céline</creator><creator>Galliez, Kévin</creator><creator>Agarande, Michelle</creator><general>Springer International Publishing</general><general>Springer</general><general>Springer Nature B.V</general><general>Springer Verlag</general><scope>AAYXX</scope><scope>CITATION</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0002-8041-2990</orcidid><orcidid>https://orcid.org/0000-0003-3829-7842</orcidid></search><sort><creationdate>20210801</creationdate><title>Quantification of curium isotopes in environmental samples: drawbacks, speciation and specific tracer</title><author>Habibi, Azza ; Le Corre, Roselyne ; Wampach Aubert, Christèle ; Fleury, Sandrine ; Hennequet, Patricia ; Augeray, Céline ; Galliez, Kévin ; Agarande, Michelle</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c436t-5a94bd26df189d9ba1bb034aace83f440f8df99a370c1a584391944cc5c290673</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Chemical Sciences</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Curium isotopes</topic><topic>Diagnostic Radiology</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>Inorganic Chemistry</topic><topic>Isotopes</topic><topic>Nuclear Chemistry</topic><topic>Nuclear energy</topic><topic>Nuclear fuel cycle</topic><topic>Nuclear industry</topic><topic>Nuclear Physics</topic><topic>Physical Chemistry</topic><topic>Speciation</topic><topic>Stability constants</topic><topic>Tracers (Biology)</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Habibi, Azza</creatorcontrib><creatorcontrib>Le Corre, Roselyne</creatorcontrib><creatorcontrib>Wampach Aubert, Christèle</creatorcontrib><creatorcontrib>Fleury, Sandrine</creatorcontrib><creatorcontrib>Hennequet, Patricia</creatorcontrib><creatorcontrib>Augeray, Céline</creatorcontrib><creatorcontrib>Galliez, Kévin</creatorcontrib><creatorcontrib>Agarande, Michelle</creatorcontrib><collection>CrossRef</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Habibi, Azza</au><au>Le Corre, Roselyne</au><au>Wampach Aubert, Christèle</au><au>Fleury, Sandrine</au><au>Hennequet, Patricia</au><au>Augeray, Céline</au><au>Galliez, Kévin</au><au>Agarande, Michelle</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Quantification of curium isotopes in environmental samples: drawbacks, speciation and specific tracer</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2021-08-01</date><risdate>2021</risdate><volume>329</volume><issue>2</issue><spage>545</spage><epage>554</epage><pages>545-554</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>In this study, drawbacks of the use of
243
Am as a tracer in order to quantify curium isotopes during a complex chemical procedure were highlighted. These drawbacks were investigated through a speciation computation simulation based on the compilation of over 50 stability constants. A new curium standard was then characterized and used to quantify a wide
244
Cm activities range in environmental samples. Obtained results were in excellent agreement with spiked activities and more consistent than those obtained when using
243
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| ispartof | Journal of radioanalytical and nuclear chemistry, 2021-08, Vol.329 (2), p.545-554 |
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| language | eng |
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| subjects | Chemical Sciences Chemistry Chemistry and Materials Science Curium isotopes Diagnostic Radiology Hadrons Heavy Ions Inorganic Chemistry Isotopes Nuclear Chemistry Nuclear energy Nuclear fuel cycle Nuclear industry Nuclear Physics Physical Chemistry Speciation Stability constants Tracers (Biology) |
| title | Quantification of curium isotopes in environmental samples: drawbacks, speciation and specific tracer |
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