Plasma catalysis application of gold nanoparticles for acetaldehyde decomposition

•Different sizes of gold nanoparticles were obtained by photocatalytic reduction.•Au/TiO2 is suitable catalyst for acetaldehyde removal in term of energy yield.•Plasma treatment doesn’t influence the surface Au atoms density.•The reaction mechanism of acetaldehyde decomposition by Au/TiO2 was propos...

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Veröffentlicht in:Chemical engineering journal (Lausanne, Switzerland : 1996) Switzerland : 1996), 2018-09, Vol.347, p.913-922
Hauptverfasser: Jia, Zixian, Ben Amar, Mounir, Yang, Dezheng, Brinza, Ovidiu, Kanaev, Andrei, Duten, Xavier, Vega-González, Arlette
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Sprache:eng
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Zusammenfassung:•Different sizes of gold nanoparticles were obtained by photocatalytic reduction.•Au/TiO2 is suitable catalyst for acetaldehyde removal in term of energy yield.•Plasma treatment doesn’t influence the surface Au atoms density.•The reaction mechanism of acetaldehyde decomposition by Au/TiO2 was proposed. The decomposition of acetaldehyde was investigated in a plasma-catalytic reactor. The gold-based catalysts were obtained by growing Au nanoparticles on silica beads or plates previously coated by a titanium oxo-alkoxy monolayer. The characterization of the synthesized catalysts was carried out by SEM, AFM and UV–Visible spectroscopy. Below an exposure time to UV of 20 min, a homogeneous surface coverage by the relatively small gold nanoparticle (R 
ISSN:1385-8947
1873-3212
DOI:10.1016/j.cej.2018.04.106