Microscopic Dynamics of Liquid Aluminum Oxide

Collective excitations have been observed in liquid aluminum oxide at high temperatures by combining a containerless sample environment with inelastic x-ray scattering. The excitation spectra show a well-defined triplet peak structure at lower wave vectors Q ($1 to 6 nanometers^{-1}$) and a single q...

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Veröffentlicht in:Science (American Association for the Advancement of Science) 2003-03, Vol.299 (5615), p.2047-2049
Hauptverfasser: Sinn, H., Glorieux, B., Hennet, L., Alatas, A., Hu, M., Alp, E. E., Bermejo, F. J., Price, D. L., M. -L. Saboungi
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Sprache:eng
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Zusammenfassung:Collective excitations have been observed in liquid aluminum oxide at high temperatures by combining a containerless sample environment with inelastic x-ray scattering. The excitation spectra show a well-defined triplet peak structure at lower wave vectors Q ($1 to 6 nanometers^{-1}$) and a single quasi-elastic peak at higher Q. The high-Q spectra are well described by kinetic theory. The low-Q spectra require a frequency-dependent viscosity and provide previously unknown experimental constraints on the behavior of liquids at the interface between atomistic and continuum theory.
ISSN:0036-8075
0193-4511
1095-9203
DOI:10.1126/science.1080950