Observation of exciton polariton condensation in a perovskite lattice at room temperature

Exciton polaritons, with extremely low effective mass 1 , are regarded as promising candidates to realize Bose–Einstein condensation in lattices for quantum simulations 2 towards room-temperature operations 3 – 8 . Along with the condensation, an efficient exciton polariton quantum simulator 9 would...

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Veröffentlicht in:Nature physics 2020-03, Vol.16 (3), p.301-306
Hauptverfasser: Su, Rui, Ghosh, Sanjib, Wang, Jun, Liu, Sheng, Diederichs, Carole, Liew, Timothy C. H., Xiong, Qihua
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Sprache:eng
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Zusammenfassung:Exciton polaritons, with extremely low effective mass 1 , are regarded as promising candidates to realize Bose–Einstein condensation in lattices for quantum simulations 2 towards room-temperature operations 3 – 8 . Along with the condensation, an efficient exciton polariton quantum simulator 9 would require a strong lattice with robust polariton trapping as well as strong intersite coupling to allow coherent quantum motion of polaritons within the lattice. A strong lattice can be characterized with a larger forbidden bandgap opening and a larger lattice bandwidth compared with the linewidth. However, exciton polaritons in such strong lattices have only been shown to condense at cryogenic temperatures 3 – 8 . Here, we report the observation of non-equilibrium exciton polariton condensation in a one-dimensional strong lead halide perovskite lattice at room temperature. Modulated by deep periodic potentials, the strong lead halide perovskite lattice exhibits a large forbidden bandgap opening up to 13.3 meV and a lattice band up to 8.5 meV wide, which are at least 10 times larger than previous systems. Above a critical density, we observe polariton condensation into p y orbital states with long-range spatial coherence at room temperature. Our result opens the route to the implementation of polariton condensates in quantum simulators at room temperature. Non-equilibrium Bose–Einstein condensation of exciton polaritons in chains of lead halide perovskite pillars can occur at room temperature. These condensates have long spatial coherence.
ISSN:1745-2473
1745-2481
1476-4636
DOI:10.1038/s41567-019-0764-5