Temperature-dependent photoemission on 1T-TiSe2: Interpretation within the exciton condensate phase model

The charge-density-wave phase transition of 1T-TiSe2 is studied by angle-resolved photoemission over a wide temperature range. An important chemical-potential shift which strongly evolves with temperature is evidenced. In the framework of the exciton condensate phase, the detailed temperature depend...

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Veröffentlicht in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2010-04, Vol.81 (15)
Hauptverfasser: Monney, Claude, Schwier, Eike, Gunnar Garnier, Michael, Didiot, Clement, Beck, Hans, Aebi, Philipp, Cercellier, Hervé, Marcus, Jacques, Battaglia, Corsin, Berger, Helmut, Titov, A.N.
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Sprache:eng
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Zusammenfassung:The charge-density-wave phase transition of 1T-TiSe2 is studied by angle-resolved photoemission over a wide temperature range. An important chemical-potential shift which strongly evolves with temperature is evidenced. In the framework of the exciton condensate phase, the detailed temperature dependence of the associated order parameter is extracted. Having a mean-field-like behavior at low temperature, it exhibits a nonzero value above the transition, interpreted as the signature of strong excitonic fluctuations, reminiscent of the pseudogap phase of high-temperature superconductors. Integrated intensity around the Fermi level is found to display a trend similar to the measured resistivity and is discussed within the model.
ISSN:1098-0121
1550-235X
DOI:10.1103/PhysRevB.81.155104