Stabilization of the second-order susceptibility induced in a sulfide chalcogenide glass by thermal poling

A second-order susceptibility χ ( 2 ) is created by the thermal poling method in a bulk sample of Ga 5 Ge 20 Sb 10 S 65 sulfide chalcogenide glass. We present experimental results focusing on the time-evolution properties of the created nonlinear layer. By cycling the poling operation on a sample, t...

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Veröffentlicht in:Journal of applied physics 2007-04, Vol.101 (8), p.084905-084905-6
Hauptverfasser: Zeghlache, H., Guignard, M., Kudlinski, A., Quiquempois, Y., Martinelli, G., Nazabal, V., Smektala, F.
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Sprache:eng
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Zusammenfassung:A second-order susceptibility χ ( 2 ) is created by the thermal poling method in a bulk sample of Ga 5 Ge 20 Sb 10 S 65 sulfide chalcogenide glass. We present experimental results focusing on the time-evolution properties of the created nonlinear layer. By cycling the poling operation on a sample, the generated second harmonic signal is improved, and the second-order nonlinearity is shown to be stable over several months. The χ ( 2 ) susceptibility profile is carefully reconstructed and its maximum value reaches 4-5 pm/V.
ISSN:0021-8979
1089-7550
DOI:10.1063/1.2719008