Order by Disorder and Energetic Selection of the Ground State in the XY Pyrochlore Antiferromagnet Er2Ti2O7. An Inelastic Neutron Scattering Study

Examples of materials where an " order by disorder " mechanism is at play to select a particular ground state are scarce. It has recently been proposed, however, that the antiferromagnetic XY pyrochlore Er 2 Ti 2 O 7 reveals a most convincing case of this mechanism, with the observation of...

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Veröffentlicht in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2014-08, Vol.90
Hauptverfasser: Petit, Sylvain, Robert, Julien, Guitteny, Solene, Bonville, Pierre, Decorse, Claudia, Ollivier, Jacques, Mutka, Hannu, Gingras, Michel J P, Mirebeau, Isabelle
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Sprache:eng
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Zusammenfassung:Examples of materials where an " order by disorder " mechanism is at play to select a particular ground state are scarce. It has recently been proposed, however, that the antiferromagnetic XY pyrochlore Er 2 Ti 2 O 7 reveals a most convincing case of this mechanism, with the observation of a spin gap at zone centers having recently been interpreted as a corroboration of this physics. Here we argue, however, that the anisotropy generated by the interaction-induced admixing between the crystal-field ground and excited levels provides for an alternative mechanism. It especially predicts the opening of a spin gap of about 15 μeV, which is of the same order of magnitude as the one observed experimentally. We report high-resolution inelastic neutron scattering data which can be well understood within this scenario.
ISSN:1098-0121
1550-235X
DOI:10.1103/PhysRevB.90.060410