Suppression of Stacking Order with Doping in 1T-TaS[sub.2−x]Se[sub.x]

In 1T-TaS[sub.2−x]Se[sub.x], the charge density wave (CDW) state features a star of David lattice that expands across layers as the system becomes commensurate upon cooling. The layers can also order along the c-axis, and different stacking orders have been proposed. Using neutron scattering on powd...

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Veröffentlicht in:Condensed matter 2023-10, Vol.8 (4)
Hauptverfasser: Philip, Sharon S, Louca, Despina, Stone, Matthew B, Kolesnikov, Alexander I
Format: Artikel
Sprache:eng
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Zusammenfassung:In 1T-TaS[sub.2−x]Se[sub.x], the charge density wave (CDW) state features a star of David lattice that expands across layers as the system becomes commensurate upon cooling. The layers can also order along the c-axis, and different stacking orders have been proposed. Using neutron scattering on powder samples, we compared the stacking order previously observed in 1T-TaS[sub.2] when the system is doped with Se. While at low temperature, a 13c layer sequence stacking was observed in TaS[sub.2]; this type of ordering was not evident with doping. Doping with Se results in a metallic state in which the Mott transition is suppressed, which may be linked to the absence of layer stacking.
ISSN:2410-3896
2410-3896
DOI:10.3390/condmat8040089