Resuspension processes controll variations of [sup.137]Cs activity concentrations in the ground-level air
The [sup.137]Cs activity concentration in the surface air between 1977 and 2007 was decreasing with an ecological half-life of 3.4 years, however, during 2007-2010 the yearly averaged [sup.137]Cs activity concentrations were almost constant. The increased atmospheric [sup.137]Cs and [sup.40]K levels...
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Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2012-08, Vol.293 (2), p.595 |
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Hauptverfasser: | , , , , , |
Format: | Artikel |
Sprache: | eng |
Online-Zugang: | Volltext |
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Zusammenfassung: | The [sup.137]Cs activity concentration in the surface air between 1977 and 2007 was decreasing with an ecological half-life of 3.4 years, however, during 2007-2010 the yearly averaged [sup.137]Cs activity concentrations were almost constant. The increased atmospheric [sup.137]Cs and [sup.40]K levels observed during the winter may be due to surface soil resuspension and radionuclide transport by winds, particularly from open agricultural areas, as confirmed by high correlation coefficient between [sup.137]Cs and [sup.40]K atmospheric levels (R = 0.84), and similar 7Cs/ K activity ratios in aerosols (0.07) and soils (0.05). Keywords Atmospheric radioactivity * Aerosols * Global fallout * Radionuclides * Soil resuspension |
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ISSN: | 0236-5731 |
DOI: | 10.1007/s10967-012-1693-2 |