Method for calculating the contribution of inelastic electron-electron scattering lifetimes of electronic states on (110) noble metal surfaces

A method for calculating the decay rate of surface states on the (110) noble metal surfaces within the GW approximation is described in detail. The band structure is described by a two-dimensional pseudo-potential model. As an example, the calculated lifetimes of surface states at the point on Cu(11...

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Veröffentlicht in:Russian physics journal 2012-04, Vol.54 (11), p.1196-1207
Hauptverfasser: Tsirkin, S. S., Eremeev, S. V.
Format: Artikel
Sprache:eng
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Zusammenfassung:A method for calculating the decay rate of surface states on the (110) noble metal surfaces within the GW approximation is described in detail. The band structure is described by a two-dimensional pseudo-potential model. As an example, the calculated lifetimes of surface states at the point on Cu(110) are presented. The calculated lifetime of the occupied state is approximately 2 times greater than that of the unoccupied state. The result obtained for the occupied surface state is in good agreement with the photoemission data.
ISSN:1064-8887
1573-9228
DOI:10.1007/s11182-012-9732-6