In situ measurements of radionuclide concentration in soil An investigation into detector properties and methods

In case of a release of radioactive nuclides into the environment it is necessary to have reliable methods to estimate the potential effect on people and the ecosystem. In this context the total activity deposited, the elemental composition and the depth distribution are of importance. An efficient in situ method to estimate the average contamination over larger areas using high purity germanium (HPGe) detectors has been developed. The method combines simulation of photon transport with measured detector properties. The total activity of 137 Cs determined from gamma-ray spectra recorded in situ are compared to results from soil sampling. Another in situ method has been developed to determine the depth distribution of a radionuclide contamination, using an array of small detectors inserted into the ground, as an alternative to the standard procedure of soil sampling. The possibility to use cadmium telluride (CdTe) detectors as well as lanthanum bromide (LaBr 3 ) detectors has been investigated. As a demonstration of the developed method the small-scale variation of the activity distributions in an area covering 350 m 2 have been measured and is compared to results obtained by other methods. At the time of the doctoral defense, the following paper was unpublished and had a status as follows: Paper 4: Submitted. Härtill 4 uppsatser Diss. (sammanfattning) Stockholm : Stockholms universitet, 2011 filosofie doktorsexamen Doctor philosophiae Degree of Doctor of Philosophy doctorat ès lettres sal FA32, AlbaNova universitetscentrum, Roslagstullsbacken 21, Stockholm Härtill 4 uppsatser Diss. (sammanfattning) Stockholm : Stockholms universitet, 2011 filosofie doktorsexamen Doctor philosophiae doctorat ès lettres In case of a release of radioactive nuclides into the environment it is necessary to have reliable methods to estimate the potential effect on people and the ecosystem. In this context the total activity deposited, the elemental composition and the depth distribution are of importance. An efficient in situ method to estimate the average contamination over larger areas using high purity germanium (HPGe) detectors has been developed. The method combines simulation of photon transport with measured detector properties. The total activity of 137 Cs determined from gamma-ray spectra recorded in situ are compared to results from soil sampling. Another in situ method has been developed to determine the depth distribution of a radionuclide contamination, using an a