Autonomous screening and optimization of battery formation and cycling procedures

A method of probing a multidimensional parameter space of battery cell test protocols is provided that includes defining a parameter space for a plurality of battery cells under test, discretizing the parameter space, collecting a preliminary set of cells being cycled to failure for sampling policies from across the parameter space and include multiple repetitions of the policy, specifying resource hyperparameters, parameter space hyperparameters, and algorithm hyperparameters, selecting a random subset of charging policies, testing the random subset of charging policies until a number of cycles required for early prediction of battery lifetime is achieved, inputting cycle data for early prediction into an early prediction algorithm to obtain early predictions, inputting the early predictions into an optimal experimental design (OED) algorithm to obtain recommendations for running at least one next test, running the recommended tests by repeating from the random subset testing step above, and validating final recommended policies.