Bosonic spinons in anisotropic triangular antiferromagnets

Anisotropic triangular antiferromagnets can host two primary spin excitations, namely, spinons and triplons. Here, we utilize polarization-resolved Raman spectroscopy to assess the statistics and dynamics of spinons in Ca 3 ReO 5 Cl 2 . We observe a magnetic Raman continuum consisting of one- and two-pair spinon-antispinon excitations as well as triplon excitations. The twofold rotational symmetry of the spinon and triplon excitations are distinct from magnons. The strong thermal evolution of spinon scattering is compatible with the bosonic spinon scenario. The quasilinear spinon hardening with decreasing temperature is envisaged as the ordering of one-dimensional topological defects. This discovery will enable a fundamental understanding of novel phenomena induced by lowering spatial dimensionality in quantum spin systems. Spinons are quasisparticles that can appear in anisotropic triangular lattices, however, probing the statistics and dynamics of such excitations is experimentally challenging. Here, Choi et al present Raman spectroscopy measurements of anisotropic triangular lattices, showing a bosonic evolution of the spinon scattering.