Electron–phonon coupling in superconducting 1T-PdTe2

We have determined the electron–phonon interaction in type II Dirac semimetallic 1T-PdTe 2 by means of helium atom scattering. While 1T-PdTe 2 is isostructural with 1T-PtTe 2 , only the former is superconductor. The difference can be traced to the substantially larger value of the electron–phonon co...

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Veröffentlicht in:NPJ 2D materials and applications 2021-02, Vol.5 (1), p.1-7, Article 25
Hauptverfasser: Anemone, Gloria, Casado Aguilar, Pablo, Garnica, Manuela, Calleja, Fabian, Al Taleb, Amjad, Kuo, Chia-Nung, Lue, Chin Shan, Politano, Antonio, Vázquez de Parga, Amadeo L., Benedek, Giorgio, Farías, Daniel, Miranda, Rodolfo
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Sprache:eng
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Zusammenfassung:We have determined the electron–phonon interaction in type II Dirac semimetallic 1T-PdTe 2 by means of helium atom scattering. While 1T-PdTe 2 is isostructural with 1T-PtTe 2 , only the former is superconductor. The difference can be traced to the substantially larger value of the electron–phonon coupling in 1T-PdTe 2 , λ  = 0.58, obtained from the Debye-Waller attenuation of the He specular peak. With this value and the surface Debye temperature, Θ D  = 106.2 K, we have figured out the superconducting critical temperature, T c  = 1.83 K given by the BCS theory, which is in good agreement with T c  = (1.95 ± 0.03) K obtained with low-temperature scanning tunneling microscopy. The value of the effective mass related to Θ D indicates that the large electron–phonon coupling in 1T-PdTe 2 is due to coupling, not only with the zone-center optical mode O 2 at 9.2 meV, as proposed in a recent theoretical study, but also with the zone-boundary acoustic mode LA. Our results suggest that the topological states of a Dirac cone play a negligible role on the onset of superconductivity.
ISSN:2397-7132
2397-7132
DOI:10.1038/s41699-021-00204-5