Magnetic ground state of the Kitaev Na_{2}Co_{2}TeO_{6} spin liquid candidate

As a candidate Kitaev material, Na_{2}Co_{2}TeO_{6} exhibits intriguing magnetism on a honeycomb lattice that is believed to be C_{3} symmetric. Here we report a neutron diffraction study of high-quality single crystals under a-axis magnetic fields. Our data support the less common notion of a magne...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Physical review research 2023-06, Vol.5 (2), p.L022045
Hauptverfasser: Weiliang Yao, Yang Zhao, Yiming Qiu, Christian Balz, J. Ross Stewart, Jeffrey W. Lynn, Yuan Li
Format: Artikel
Sprache:eng
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:As a candidate Kitaev material, Na_{2}Co_{2}TeO_{6} exhibits intriguing magnetism on a honeycomb lattice that is believed to be C_{3} symmetric. Here we report a neutron diffraction study of high-quality single crystals under a-axis magnetic fields. Our data support the less common notion of a magnetic ground state that corresponds to a triple-q magnetic structure with C_{3} symmetry, rather than the multidomain zigzag structure typically assumed in prototype Kitaev spin liquid candidates. In particular, we find that the field is unable to repopulate the supposed zigzag domains, where the only alternative explanation is that the domains are strongly pinned by hitherto unidentified structural reasons. If the triple-q structure is correct, then this requires reevaluation of many candidate Kitaev materials. We also find that fields beyond about 10 Tesla suppress the long-range antiferromagnetic order, allowing magnetic behavior to emerge different from that expected for a spin liquid.
ISSN:2643-1564
DOI:10.1103/PhysRevResearch.5.L022045