Heavy fermion behavior in the quasi-one-dimensional Kondo lattice CeCo2Ga8
Dimensionality plays an essential role in determining the anomalous non-Fermi liquid properties in heavy fermion systems. So far most heavy fermion compounds are quasi-two-dimensional or three-dimensional. Here we report the synthesis and systematic investigations of the single crystals of the quasi...
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Veröffentlicht in: | npj quantum materials 2017-07, Vol.2 (1), p.1-6, Article 36 |
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Zusammenfassung: | Dimensionality plays an essential role in determining the anomalous non-Fermi liquid properties in heavy fermion systems. So far most heavy fermion compounds are quasi-two-dimensional or three-dimensional. Here we report the synthesis and systematic investigations of the single crystals of the quasi-one-dimensional Kondo lattice CeCo
2
Ga
8
. Resistivity measurements at ambient pressure reveal the onset of coherence at
T
* ≈ 20 K and non-Fermi liquid behavior with linear temperature dependence over a decade in temperature from 2 to 0.1 K. The specific heat increases logarithmically with lowering temperature between 10 and 2 K and reaches 800 mJ/mol K
2
at 1 K, suggesting that CeCo
2
Ga
8
is a heavy fermion compound in the close vicinity of a quantum critical point. Resistivity measurements under pressure further confirm the non-Fermi liquid behavior in a large temperature–pressure range. The magnetic susceptibility is found to follow the typical behavior for a one-dimensional spin chain from 300 K down to
T
*, and first-principles calculations predict flat Fermi surfaces for the itinerant
f
-electron bands. These suggest that CeCo
2
Ga
8
is a rare example of the quasi-one-dimensional Kondo lattice, but its non-Fermi liquid behaviors resemble those of the quasi-two-dimensional YbRh
2
Si
2
family. The study of the quasi-one-dimensional CeCo
2
Ga
8
family may therefore help us to understand the role of dimensionality on heavy fermion physics and quantum criticality.
Heavy fermion materials: evidence for a quasi-one-dimensional Kondo lattice
Evidence is provided for a heavy fermion material that is an unusual example of a quasi-one-dimensional Kondo lattice system. Heavy fermion materials are compounds with localised magnetic moments that interact strongly with the surrounding conduction electrons, causing a rich variety of exotic behaviour to arise. And when these moments form a periodic array, a Kondo lattice can be formed —where scattering off the moments becomes coherent. An international team of researchers led by Yi-feng Yang and Youguo Shi from the Institute of Physics, Chinese Academy of Sciences now present an unusual example of a Kondo lattice system that is quasi-one-dimensional in nature. Using a combination of experiments and first-principles calculations they show that the cerium atoms in single crystals of CeCo
2
Ga
8
form chains, leading to quasi-one-dimensional Kondo lattice behaviour and unusual quantum critical scalings that are not expect |
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ISSN: | 2397-4648 2397-4648 |
DOI: | 10.1038/s41535-017-0040-9 |