High spin ↔ low spin ultrafast excitation and relaxation of an isolated iron(II) complex

High spin ↔ low spin ultrafast excitation and relaxation of an isolated iron(II) complex

Picosecond and femtosecond time resolved pump-probe experiments make it possible to study both the low spin (LS) to high spin (HS) and high spin to low spin excitation and relaxation processes in the same isolated iron(II) complex. We demonstrate that both LS arrow right HS and HS arrow right LS can...

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Veröffentlicht in:EPJ Web of conferences 2013-01, Vol.41, p.5010-np
Hauptverfasser: Galle, G., Tribollet, J., Jonusauskas, G., Tondusson, M., Mauriac, C., Létard, J.F., Freysz, E.
Format: Artikel
Sprache:eng
Schlagworte:
Excitation
Femtosecond
Optics
Physics
Pumps
Time
Time resolved
Wavelengths
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Zusammenfassung:Picosecond and femtosecond time resolved pump-probe experiments make it possible to study both the low spin (LS) to high spin (HS) and high spin to low spin excitation and relaxation processes in the same isolated iron(II) complex. We demonstrate that both LS arrow right HS and HS arrow right LS can be recorded by changing the pump wavelength and occur on the same time scale.
ISSN:2100-014X
2100-014X
DOI:10.1051/epjconf/20134105010