Thinfilm Hybrid Nanostructures: A Perspective to Subcycle Opto-Electronics and Coherent Control

In this article we present a theoretical investigation of gold-silica-silver nanostructures and their optical properties with respect to ultrafast electronic applications and coherent control by tailored optical fields. We found a remarkable sensitive behavior to the carrier envelope phase (CEP) of the driving laser pulses in the coupling of surface and bulk plasmons leading to a superposition of distinct modes with a time-dependent amplitude structure. Furthermore, we show a rather complex temporal evolution of plasmonic surface modes. Our results suggest the potential for coherent control of the time-dependent resonant coupling between surface and volume modes by tailored laser pulses and foster the field of time-dependent spectroscopy of thinfilm hybrid nanostructures with single layer thickness down to the two-dimensional limit.