Model simulations of atmospheric methane (1997–2016) and their evaluation using NOAA and AGAGE surface and IAGOS-CARIBIC aircraft observations

Methane (CH.sub.4) is an important greenhouse gas, and its atmospheric budget is determined by interacting sources and sinks in a dynamic global environment. Methane observations indicate that after almost a decade of stagnation, from 2006, a sudden and continuing global mixing ratio increase took p...

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Veröffentlicht in:Atmospheric chemistry and physics 2020-05, Vol.20 (9), p.5787-5809
Hauptverfasser: Zimmermann, Peter H, Brenninkmeijer, Carl A. M, Pozzer, Andrea, Jöckel, Patrick, Winterstein, Franziska, Zahn, Andreas, Houweling, Sander, Lelieveld, Jos
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Sprache:eng
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Zusammenfassung:Methane (CH.sub.4) is an important greenhouse gas, and its atmospheric budget is determined by interacting sources and sinks in a dynamic global environment. Methane observations indicate that after almost a decade of stagnation, from 2006, a sudden and continuing global mixing ratio increase took place. We applied a general circulation model to simulate the global atmospheric budget, variability, and trends of methane for the period 1997-2016. Using interannually constant CH.sub.4 a priori emissions from 11 biogenic and fossil source categories, the model results are compared with observations from 17 Advanced Global Atmospheric Gases Experiment (AGAGE) and National Oceanic and Atmospheric Administration (NOAA) surface stations and intercontinental Civil Aircraft for the Regular observation of the atmosphere Based on an Instrumented Container (CARIBIC) flights, with > 4800 CH.sub.4 samples, gathered on > 320 flights in the upper troposphere and lowermost stratosphere.
ISSN:1680-7324
1680-7316
1680-7324
DOI:10.5194/acp-20-5787-2020