Evaluation of dosimetric characteristics of a ternary nanocomposite based on High Density Polyethylene/Bismuth Oxide/Graphene Oxide for gamma-rays

This research aims to investigate a ternary nanocomposite based on High Density Polyethylene/ Bismuth Oxide/Graphene Oxide (HDPE/Bi 2 O 3 /GO) at various concentrations. Solution method was used to fabricate the samples. FESEM-EDX mapping, AFM, TEM, XRD, XPS, FTIR, and TGA/DTG analyses were carried...

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Veröffentlicht in:Scientific reports 2022-11, Vol.12 (1), p.18798-17, Article 18798
Hauptverfasser: Veiskarami, Amir, Sardari, Dariush, Malekie, Shahryar, Mofrad, Farshid Babapour, Kashian, Sedigheh
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Sprache:eng
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Zusammenfassung:This research aims to investigate a ternary nanocomposite based on High Density Polyethylene/ Bismuth Oxide/Graphene Oxide (HDPE/Bi 2 O 3 /GO) at various concentrations. Solution method was used to fabricate the samples. FESEM-EDX mapping, AFM, TEM, XRD, XPS, FTIR, and TGA/DTG analyses were carried out on the samples. XRD analysis demonstrated a semi-crystalline behavior for the samples. TEM analysis exhibited a cauliflower-like structure of the material. The sample was irradiated by gamma-rays of 60 Co source over the dose rate of 30–254 mGy/min and the electric current was measured as the response of the real-time dosimeter. Thus, various dosimetric characteristics were performed, namely linearity, angular dependence, energy dependence, bias-polarity, field size, and repeatability of the data. Results showed that response of the dosimeter was linear in the range of the investigated dose rate. The sensitivity of the 60 wt% Bi 2 O 3 sample was measured as 3.4 nC·mGy −1 . The angular response variation was 20% for normal beam incidence. The response of the dosimeter to assess the energy dependency was obtained as 2.2% at the radiation field of the 137 Cs and 60 Co beams. The dosimeter response was dependent on the bias-polarity, with maximum discrepancy of 11.1%. The dosimetry response was highly dependent upon the radiation field size. The repeatability of the dosimeter response was measured with standard deviation less than 1%. As well, the dosimeter response during the one-hour irradiation was stable with a standard deviation of 0.66%. Results showed that considering some correction factors, this material can be used for dosimetry of gamma-rays at the therapy level.
ISSN:2045-2322
2045-2322
DOI:10.1038/s41598-022-23605-y